The goal of Project ATLANTA is to derive a better scientific understanding of how land cover changes associated with urbanization affect climate and air quality. In this project the role that clouds play in this relationship was studied. Through GOES satellite observations and RAMS modeling of the Atlanta area, we found that in Atlanta (1) clouds are more frequent than in the surrounding rural areas; (2) clouds cool the surface by shading and thus tend to counteract the warming effect of urbanization; (3) clouds reflect sunlight, which might other wise be used to produce ozone; and (4) clouds decrease biogenic emission of ozone precursors, and they probably decrease ozone concentration. We also found that mesoscale modeling of clouds, especially of small, summertime clouds, needs to be improved and that coupled mesoscale and air quality models are needed to completely understand the mediating role that clouds play in the relationship between land use/land cover change and the climate and air quality of Atlanta. It is strongly recommended that more cities be studied to strengthen and extend these results.